18 research outputs found

    n_TOF: Measurements of Key Reactions of Interest to AGB Stars

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    In the last 20 years, the neutron time-of-flight facility n_TOF at CERN has been providing relevant data for the astrophysical slow neutron capture process (s process). At n_TOF, neutron-induced radiative capture (n,γ) as well as (n,p) and (n,α) reaction cross sections are measured as a function of energy, using the time-of-flight method. Improved detection systems, innovative ideas and collaborations with other neutron facilities have lead to a considerable contribution of the n_TOF collaboration to studying the s process in asymptotic giant branch stars. Results have been reported for stable and radioactive samples, i.e.,24,25,26Mg,26Al,33S,54,57Fe,58,59,62,63Ni,70,72,73Ge,90,91,92,93,94,96Zr,139La,140Ce,147Pm,151Sm,154,155,157Gd,171Tm,186,187,188Os,197Au,203,204Tl,204,206,207Pb and209Bi isotopes, while others are being studied or planned to be studied in the near future. In this contribution, we present an overview of the most successful achievements, and an outlook of future challenging measurements, including ongoing detection system developments

    Conceptual design of the early implementation of the NEutron Detector Array (NEDA) with AGATA

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    The NEutron Detector Array (NEDA) project aims at the construction of a new high-efficiency compact neutron detector array to be coupled with large (Formula presented.) -ray arrays such as AGATA. The application of NEDA ranges from its use as selective neutron multiplicity filter for fusion-evaporation reaction to a large solid angle neutron tagging device. In the present work, possible configurations for the NEDA coupled with the Neutron Wall for the early implementation with AGATA has been simulated, using Monte Carlo techniques, in order to evaluate their performance figures. The goal of this early NEDA implementation is to improve, with respect to previous instruments, efficiency and capability to select multiplicity for fusion-evaporation reaction channels in which 1, 2 or 3 neutrons are emitted. Each NEDA detector unit has the shape of a regular hexagonal prism with a volume of about 3.23l and it is filled with the EJ301 liquid scintillator, that presents good neutron- (Formula presented.) discrimination properties. The simulations have been performed using a fusion-evaporation event generator that has been validated with a set of experimental data obtained in the 58Ni + 56Fe reaction measured with the Neutron Wall detector array

    First Results of the 140^{140}Ce(n,γ)141^{141}Ce Cross-Section Measurement at n_TOF

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    An accurate measurement of the 140^{140}Ce(n,γ) energy-dependent cross-section was performed at the n_TOF facility at CERN. This cross-section is of great importance because it represents a bottleneck for the s-process nucleosynthesis and determines to a large extent the cerium abundance in stars. The measurement was motivated by the significant difference between the cerium abundance measured in globular clusters and the value predicted by theoretical stellar models. This discrepancy can be ascribed to an overestimation of the 140^{140}Ce capture cross-section due to a lack of accurate nuclear data. For this measurement, we used a sample of cerium oxide enriched in 140^{140}Ce to 99.4%. The experimental apparatus consisted of four deuterated benzene liquid scintillator detectors, which allowed us to overcome the difficulties present in the previous measurements, thanks to their very low neutron sensitivity. The accurate analysis of the p-wave resonances and the calculation of their average parameters are fundamental to improve the evaluation of the 140^{140}Ce Maxwellian-averaged cross-section

    First Results of the 140^{140}Ce(n,γ)141^{141}Ce Cross-Section Measurement at n_TOF

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    An accurate measurement of the 140^{140}Ce(n,γ) energy-dependent cross-section was performed at the n_TOF facility at CERN. This cross-section is of great importance because it represents a bottleneck for the s-process nucleosynthesis and determines to a large extent the cerium abundance in stars. The measurement was motivated by the significant difference between the cerium abundance measured in globular clusters and the value predicted by theoretical stellar models. This discrepancy can be ascribed to an overestimation of the 140^{140}Ce capture cross-section due to a lack of accurate nuclear data. For this measurement, we used a sample of cerium oxide enriched in 140^{140}Ce to 99.4%. The experimental apparatus consisted of four deuterated benzene liquid scintillator detectors, which allowed us to overcome the difficulties present in the previous measurements, thanks to their very low neutron sensitivity. The accurate analysis of the p-wave resonances and the calculation of their average parameters are fundamental to improve the evaluation of the 140^{140}Ce Maxwellian-averaged cross-section

    Mortality from gastrointestinal congenital anomalies at 264 hospitals in 74 low-income, middle-income, and high-income countries: a multicentre, international, prospective cohort study

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    Summary Background Congenital anomalies are the fifth leading cause of mortality in children younger than 5 years globally. Many gastrointestinal congenital anomalies are fatal without timely access to neonatal surgical care, but few studies have been done on these conditions in low-income and middle-income countries (LMICs). We compared outcomes of the seven most common gastrointestinal congenital anomalies in low-income, middle-income, and high-income countries globally, and identified factors associated with mortality. Methods We did a multicentre, international prospective cohort study of patients younger than 16 years, presenting to hospital for the first time with oesophageal atresia, congenital diaphragmatic hernia, intestinal atresia, gastroschisis, exomphalos, anorectal malformation, and Hirschsprung’s disease. Recruitment was of consecutive patients for a minimum of 1 month between October, 2018, and April, 2019. We collected data on patient demographics, clinical status, interventions, and outcomes using the REDCap platform. Patients were followed up for 30 days after primary intervention, or 30 days after admission if they did not receive an intervention. The primary outcome was all-cause, in-hospital mortality for all conditions combined and each condition individually, stratified by country income status. We did a complete case analysis. Findings We included 3849 patients with 3975 study conditions (560 with oesophageal atresia, 448 with congenital diaphragmatic hernia, 681 with intestinal atresia, 453 with gastroschisis, 325 with exomphalos, 991 with anorectal malformation, and 517 with Hirschsprung’s disease) from 264 hospitals (89 in high-income countries, 166 in middleincome countries, and nine in low-income countries) in 74 countries. Of the 3849 patients, 2231 (58·0%) were male. Median gestational age at birth was 38 weeks (IQR 36–39) and median bodyweight at presentation was 2·8 kg (2·3–3·3). Mortality among all patients was 37 (39·8%) of 93 in low-income countries, 583 (20·4%) of 2860 in middle-income countries, and 50 (5·6%) of 896 in high-income countries (p<0·0001 between all country income groups). Gastroschisis had the greatest difference in mortality between country income strata (nine [90·0%] of ten in lowincome countries, 97 [31·9%] of 304 in middle-income countries, and two [1·4%] of 139 in high-income countries; p≤0·0001 between all country income groups). Factors significantly associated with higher mortality for all patients combined included country income status (low-income vs high-income countries, risk ratio 2·78 [95% CI 1·88–4·11], p<0·0001; middle-income vs high-income countries, 2·11 [1·59–2·79], p<0·0001), sepsis at presentation (1·20 [1·04–1·40], p=0·016), higher American Society of Anesthesiologists (ASA) score at primary intervention (ASA 4–5 vs ASA 1–2, 1·82 [1·40–2·35], p<0·0001; ASA 3 vs ASA 1–2, 1·58, [1·30–1·92], p<0·0001]), surgical safety checklist not used (1·39 [1·02–1·90], p=0·035), and ventilation or parenteral nutrition unavailable when needed (ventilation 1·96, [1·41–2·71], p=0·0001; parenteral nutrition 1·35, [1·05–1·74], p=0·018). Administration of parenteral nutrition (0·61, [0·47–0·79], p=0·0002) and use of a peripherally inserted central catheter (0·65 [0·50–0·86], p=0·0024) or percutaneous central line (0·69 [0·48–1·00], p=0·049) were associated with lower mortality. Interpretation Unacceptable differences in mortality exist for gastrointestinal congenital anomalies between lowincome, middle-income, and high-income countries. Improving access to quality neonatal surgical care in LMICs will be vital to achieve Sustainable Development Goal 3.2 of ending preventable deaths in neonates and children younger than 5 years by 2030

    New radiative neutron capture measurement of 207Pb and 209Bi

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    This new measurement of the (n, ) capture cross sections of 207Pb and 209Bi has been motivated by i) the aim to achieve a better understanding of the s-process stellar nucleosynthesis in its termination region and ii) the design of accelerator driven systems (ADS) based on a lead-bismuth eutectic spallation core. The measurement has been performed using the total energy detector technique, since the lower neutron sensitivity achievable with such a detection system represents a clear advantage versus the alternative total absorption method. However, the former technique has been a source of controversy between experimentalists and therefore, an important part of the present work has been dedicated rst to the review and further development of the so called Pulse Height Weighting Technique (PHWT). Performing dedicated measurements at the CERN n TOF installation we have experimentally validated this technique, determining that a systematic uncertainty better than 2% can be achieved. Once the measuring technique has been demonstrated to be well under control, the measurement of the radiative capture cross section of 207Pb and 209Bi was carried out. Experimental sources of systematic uncertainty have been thoroughly treated by means of Monte Carlo simulations. An R-matrix analysis of the resolved resonance region has been performed for both nuclides, deriving the total resonance radiative capture cross section and resonance parameters where possible. Previous measurements of these isotopes were aected by large systematic corrections mainly due to the neutron sensitivity of the detection system used. In the present work these isotopes have been measured by employing an optimized detection setup, which permitted the determination of their cross sections with a practically negligible neutron sensitivity deviation. A comparison between the results obtained here and current evaluated data les is also presented, revealing high deviations mainly on s-wave resonances. These are to be ascribed to the high systematic uncertainty of the previous measurements, in which these evaluations are based. Implications of the new results in the eld of stellar nucleosynthesis as well as in ADS engineering are studied and discussed

    Prospects for direct neutron capture measurements on s-process branching point isotopes

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    The neutron capture cross sections of several unstable key isotopes acting as branching points in the s-process are crucial for stellar nucleosynthesis studies, but they are very challenging to measure directly due to the difficult production of sufficient sample material, the high activity of the resulting samples, and the actual (n, γ) measurement, where high neutron fluxes and effective background rejection capabilities are required. At present there are about 21 relevant s-process branching point isotopes whose cross section could not be measured yet over the neutron energy range of interest for astrophysics. However, the situation is changing with some very recent developments and upcoming technologies. This work introduces three techniques that will change the current paradigm in the field: the use of γ-ray imaging techniques in (n, γ) experiments, the production of moderated neutron beams using high-power lasers, and double capture experiments in Maxwellian neutron beams
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